ACCURATE TIME-DEPENDENT WAVE PACKET STUDY OF THE H++LiH REACTION AT EARLY UNIVERSE CONDITIONS
  
Yazarlar (6)
Prof. Dr. Emine TANIŞ Kırşehir Ahi Evran Üniversitesi, Türkiye
Niyazi Bulut
Fırat Üniversitesi, Türkiye
Castillo Jesus Fernandez
Banares Luis
Aoiz F Javier
Roncero Octavio
Makale Türü Açık Erişim Özgün Makale (SSCI, AHCI, SCI, SCI-Exp dergilerinde yayınlanan tam makale)
Dergi Adı The Astrophysical Journal
Dergi ISSN 0004-637X Wos Dergi Scopus Dergi
Dergi Tarandığı Indeksler SCI-Expanded
Makale Dili İngilizce Basım Tarihi 10-2012
Cilt / Sayı / Sayfa 759 / 1 / 31– DOI 10.1088/0004-637X/759/1/31
Makale Linki http://dx.doi.org/10.1088/0004-637x/759/1/31
Özet
The dynamics and kinetics of the H++ LiH reaction have been studied using a quantum reactive time-dependent wave packet (TDWP) coupled-channel quantum mechanical method on an ab initio potential energy surface at conditions of the early universe. The total reaction probabilities for the H++ LiH (v= 0, j= 0)→ H+ 2+ Li process have been calculated from 5× 10− 3 eV up to 1 eV for total angular momenta J from 0 to 110. Using a Langevin model, integral cross sections have been calculated in that range of collision energies and extrapolated for energies below 5× 10− 3 eV. The calculated rate constants are found to be nearly independent of temperature in the 10–1000 K interval with a value of≈ 10− 9 cm 3 s− 1, which is in good agreement with estimates used in evolutionary models of the early universe lithium chemistry.
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